Multi-residue analysis of traces of pesticides and antibiotics in honey by HPLC-MS-MS

Anal Bioanal Chem. 2008 Jun;391(3):1011-20. doi: 10.1007/s00216-008-2003-2. Epub 2008 Apr 20.

Abstract

The aim of this work was to develop an analytical method for simultaneous assay of residues of two families of antibiotics, and three pesticides, in honey. The assays involved a mixture of five tetracyclines, four sulfamides, and the pesticides coumaphos, carbendazim, and amitraz (two metabolites). All the compounds were extracted from honey and pre-concentrated by optimised solid-phase extraction (SPE). Analysis was by high-performance liquid chromatography-mass spectrometry-mass spectrometry (HPLC-MS-MS) using a triple-quadrupole spectrometer in multiple reaction monitoring (MRM) mode in order to identify and quantify the compounds present (Sheth et al J Agric Food Chem 38:1125-1130, 1990). During development of the analytical method a strong matrix effect was found that depended on the floral origin of the honey. This led to the development of a standard additions method to quantify the contaminants sought.

Publication types

  • Validation Study

MeSH terms

  • Anti-Bacterial Agents / analysis*
  • Chromatography, High Pressure Liquid / instrumentation
  • Chromatography, High Pressure Liquid / methods
  • Honey / analysis*
  • Molecular Structure
  • Pesticides / analysis*
  • Reproducibility of Results
  • Solid Phase Extraction / methods
  • Tandem Mass Spectrometry / instrumentation
  • Tandem Mass Spectrometry / methods*

Substances

  • Anti-Bacterial Agents
  • Pesticides