Fixure-reduce method for the synthesis of Cu2O/MWCNTs nanocomposites and its application as enzyme-free glucose sensor

Biosens Bioelectron. 2009 Jul 15;24(11):3395-8. doi: 10.1016/j.bios.2009.04.031. Epub 2009 May 3.

Abstract

Cu(2)O/MWCNT (multi-walled carbon nanotubes) nanocomposites were successfully prepared in large quantities with a new fixure-reduction method under low temperature. The morphology and shape of the Cu(2)O/MWCNTs nanocomposites were characterized by field emission scanning electron microscopes (FESEMs), energy dispersive X-ray (EDX), X-ray photoelectron spectroscopy (XPS) and X-ray powder diffraction (XRD), respectively. Cyclic voltammetry (CV) was used to evaluate the electrochemical performance of the Cu(2)O/MWCNTs nanocomposites modified electrode towards glucose. Compared to the bare GCE, the Cu(2)O nanoparticles and the MWCNTs modified electrode, the Cu(2)O/MWCNTs modified electrode displays high electrocatalytic activity towards the oxidation of glucose. With a potential of -0.20 V, the Cu(2)O/MWCNTs modified electrode was used to determine glucose by amperometric, showing significantly lower overvoltage and a linear dependence (R=0.9958) in the concentration up to 10 microM with a sensitivity of 6.53 microA micromol L(-1) and a detection limit of 0.05 micromol L(-1) (signal-to-noise ratio of 3). In summary, the preparation process of the nanocomposites is very simple and the nanocomposites could be used for the development of enzyme-free glucose sensor.

Publication types

  • Evaluation Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Biosensing Techniques / instrumentation*
  • Copper / chemistry*
  • Electrochemistry / instrumentation*
  • Electrodes
  • Enzymes / chemistry
  • Equipment Design
  • Equipment Failure Analysis
  • Glucose / analysis*
  • Manufactured Materials
  • Nanotechnology / instrumentation*
  • Nanotubes, Carbon / chemistry*
  • Nanotubes, Carbon / ultrastructure
  • Oxidation-Reduction
  • Transducers

Substances

  • Enzymes
  • Nanotubes, Carbon
  • Copper
  • Glucose
  • cupric oxide