Abstract
In this study we showed that Rottlerin (also called Kamala or Mallotoxin), a natural product purified from Mallotus phillippinensis, is a potent suppressor of human keratinocytes (HaCaT cell line) proliferation. Following Rottlerin treatment, Thymidine incorporation into DNA and re-epithelialisation in a scratch wound model was decreased. At the molecular level, Rottlerin hampered the NFkB activation process, causing loss of cyclin D1 and promoting, in a PKCdelta-dependent pathway, ERK activation, which, in turn induced the cell cycle inhibitor p21 Cip1/Kip1. The NFkB-dependent drop in cyclin D1, along with the PKCdelta/ERK-dependent induction of p21 Cip1/Kip1, is responsible for growth arrest. These results open the way to further investigation on the Rottlerin therapeutic potential against keratinocyte hyper-proliferative disorders.
Publication types
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Research Support, Non-U.S. Gov't
MeSH terms
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Acetophenones / pharmacology*
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Active Transport, Cell Nucleus / drug effects
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Benzopyrans / pharmacology*
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Cell Cycle / drug effects
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Cell Line, Transformed / drug effects
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Cells, Cultured / cytology
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Cells, Cultured / drug effects
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Cyclin D1 / biosynthesis
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Cyclin D2
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Cyclin-Dependent Kinase Inhibitor p21 / biosynthesis
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Cyclin-Dependent Kinase Inhibitor p21 / genetics
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Cyclins / biosynthesis
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Cyclins / genetics
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Drug Evaluation, Preclinical
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Extracellular Signal-Regulated MAP Kinases / antagonists & inhibitors
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Extracellular Signal-Regulated MAP Kinases / metabolism
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Gene Expression Regulation / drug effects
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Genes, bcl-1 / drug effects
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Growth Inhibitors / pharmacology*
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Humans
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In Vitro Techniques
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Keratinocytes / cytology
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Keratinocytes / drug effects*
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NF-kappa B / antagonists & inhibitors
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Phosphorylation / drug effects
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Protein Kinase C-delta / antagonists & inhibitors
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Protein Kinase C-delta / physiology
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Protein Kinase Inhibitors / pharmacology*
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Protein Processing, Post-Translational / drug effects
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Wound Healing / drug effects
Substances
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Acetophenones
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Benzopyrans
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CCND1 protein, human
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CCND2 protein, human
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CDKN1A protein, human
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Cyclin D2
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Cyclin-Dependent Kinase Inhibitor p21
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Cyclins
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Growth Inhibitors
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NF-kappa B
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Protein Kinase Inhibitors
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Cyclin D1
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rottlerin
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Protein Kinase C-delta
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Extracellular Signal-Regulated MAP Kinases