Discovery of orally bioavailable imidazo[1,2-a]pyrazine-based Aurora kinase inhibitors

Bioorg Med Chem Lett. 2010 Nov 15;20(22):6739-43. doi: 10.1016/j.bmcl.2010.08.140. Epub 2010 Sep 18.

Abstract

We report a series of potent imidazo[1,2-a]pyrazine-based Aurora kinase inhibitors. Optimization of the solvent accessible 8-position led to improvements in both oral bioavailability and off-target kinase inhibition. Compound 25 demonstrates anti-tumor activity in an A2780 ovarian tumor xenograft model.

MeSH terms

  • Administration, Oral
  • Animals
  • Aurora Kinases
  • Biological Availability
  • Cell Line, Tumor
  • Female
  • Humans
  • Imidazoles / chemistry
  • Imidazoles / pharmacokinetics
  • Imidazoles / pharmacology*
  • Protein Kinase Inhibitors / chemistry
  • Protein Kinase Inhibitors / pharmacokinetics
  • Protein Kinase Inhibitors / pharmacology*
  • Protein Serine-Threonine Kinases / antagonists & inhibitors*
  • Pyrazines / chemistry
  • Pyrazines / pharmacokinetics
  • Pyrazines / pharmacology*
  • Xenograft Model Antitumor Assays

Substances

  • Imidazoles
  • Protein Kinase Inhibitors
  • Pyrazines
  • imidazo(1,2-a)pyrazine
  • Aurora Kinases
  • Protein Serine-Threonine Kinases