A novel truncated basic fibroblast growth factor fragment-conjugated poly (ethylene glycol)-cholesterol amphiphilic polymeric drug delivery system for targeting to the FGFR-overexpressing tumor cells

Int J Pharm. 2011 Apr 15;408(1-2):173-82. doi: 10.1016/j.ijpharm.2011.01.042. Epub 2011 Jan 26.

Abstract

Targeted uptake of therapeutic nanoparticles in tumor cells-specific manner represents a potentially powerful technology in cancer therapy. In present study, we proposed a drug delivery system formulated with biocompatible and biodegradable cholesterol-block-poly (ethylene glycol) (Chol-PEG(2000)-COOH) polymer. And the surface of the polymer was chemically linked with truncated bFGF fragments (tbFGF). The tbFGF could recognize fibroblast growth factor receptors (FGFR) that are highly expressed by a variety of human cancer cells. The micelles had a size distribution of about 10-50 nm and significantly enhanced the cytotoxicity of paclitaxel to LL/2 cells as demonstrated by MTT test (IC₅₀=0.21 μg/mL for tbFGF conjugated Chol-PEG(2000)-COOH micelles (tbFGF-M-PTX) versus 26.43 μg/mL for free paclitaxel, respectively). Flow cytometry revealed the cellular uptake of rhodamine B encapsulated in the tbFGF-conjugated micelles was increased by 6.6-fold for HepG2, 6.2-fold for A549, 2.9-fold for C26 and 2.7-fold for LL/2 tumor cells, respectively, compared with micelles without tbFGF. The fluorescence spectroscopy images further demonstrated that the tbFGF conjugated micelles could specifically bind to the tumor cells that over-expressed FGFRs and then release rhodamine B into the cytoplasm. Our results suggest the tbFGF conjugated Chol-PEG(2000)-COOH micelles have great potential application for tumor targeting therapy.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Antineoplastic Agents / administration & dosage*
  • Cell Line, Tumor
  • Cell Survival / drug effects
  • Chemistry, Pharmaceutical
  • Cholesterol / analogs & derivatives*
  • Cholesterol / chemical synthesis
  • Cholesterol / chemistry
  • Cytoplasm / drug effects
  • Cytoplasm / metabolism
  • Drug Carriers / chemical synthesis
  • Drug Carriers / chemistry*
  • Electrophoresis, Polyacrylamide Gel
  • Fibroblast Growth Factor 2 / administration & dosage*
  • Humans
  • Mice
  • Micelles
  • Microscopy, Atomic Force
  • Microscopy, Electron, Transmission
  • Microscopy, Fluorescence
  • Molecular Structure
  • Particle Size
  • Peptide Fragments / administration & dosage*
  • Polyethylene Glycols / chemical synthesis
  • Polyethylene Glycols / chemistry*
  • Protein Binding
  • Receptors, Fibroblast Growth Factor / antagonists & inhibitors*
  • Receptors, Fibroblast Growth Factor / biosynthesis
  • Solubility
  • Surface Properties
  • Surface-Active Agents / chemical synthesis
  • Surface-Active Agents / chemistry*

Substances

  • Antineoplastic Agents
  • Drug Carriers
  • Micelles
  • Peptide Fragments
  • Receptors, Fibroblast Growth Factor
  • Surface-Active Agents
  • polyethylene glycol-cholesterol
  • Fibroblast Growth Factor 2
  • Polyethylene Glycols
  • Cholesterol