Performance enhancement of fullerene-based solar cells by light processing

Nat Commun. 2013:4:2227. doi: 10.1038/ncomms3227.

Abstract

A key challenge to the commercialization of organic bulk heterojunction solar cells is the achievement of morphological stability, particularly under thermal stress conditions. Here we show that a low-level light exposure processing step during fabrication of blend polymer:PC60BM solar cells can result in a 10-fold increase in device thermal stability and, under certain conditions, enhanced device performance. The enhanced stability is linked to the light-induced oligomerization of PC60BM that effectively hinders their diffusion and crystallization in the blend. We thus suggest that light processing may be a promising, general and cost-effective strategy to optimize fullerene-based solar cell performance. The low level of light exposure required suggests not only that this may be an easily implementable strategy to enhance performance, but also that light-induced PC60BM oligomerization may have inadvertently influenced previous studies of organic solar cell device behaviour.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Crystallization
  • Fullerenes / chemistry*
  • Humans
  • Light
  • Polymerization
  • Solar Energy / statistics & numerical data*
  • Thiadiazoles / chemistry*

Substances

  • Fullerenes
  • Thiadiazoles