Quantification of central substance P receptor occupancy by aprepitant using small animal positron emission tomography

Int J Neuropsychopharmacol. 2014 Oct 31;18(2):pyu030. doi: 10.1093/ijnp/pyu030.

Abstract

Background: Central substance P receptors, termed NK-1 receptors, have been considered as therapeutic targets in the development of drugs against diverse conditions, including emesis, overactive bladder, and depression.

Methods: Here, we applied small animal positron emission tomography (PET) and a radioligand for NK-1 receptors ([(18)F]FE-SPA-RQ) for measuring occupancies of these receptors by a selective antagonist (aprepitant) in order to examine the validity of this in vivo imaging system for preclinical characterization of candidate agents acting on NK-1 receptors, and as a tool for predicting optimal doses in humans.

Results: PET in gerbils depicted high uptake in the striatum and dose-dependent displacement with increasing doses of aprepitant. Occupancies increased as a function of aprepitant plasma concentrations according to a one-site competition model, which agrees with reported occupancy-concentration relationships in clinical studies after correction for species differences in plasma protein-unbound aprepitant fractions. These occupancy data were further supported by ex vivo autoradiography of brain samples from aprepitant-treated gerbils. In a pilot study of a marmoset, we obtained more accurate determinations of NK-1 receptor occupancy, less affected by spillover of signals from extracranial tissues than in gerbil experiments.

Conclusions: These findings support the utility of small animals and quantitative PET in the development of drugs targeting NK-1 receptors.

Keywords: NK-1 receptor; receptor occupancy; small-animal PET; substance P.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Aprepitant
  • Autoradiography
  • Brain / diagnostic imaging
  • Brain / drug effects*
  • Brain / metabolism*
  • Callithrix
  • Dose-Response Relationship, Drug
  • Gerbillinae
  • Humans
  • Male
  • Morpholines / pharmacokinetics*
  • Neurokinin-1 Receptor Antagonists / pharmacokinetics*
  • Pilot Projects
  • Positron-Emission Tomography / methods
  • Receptors, Neurokinin-1 / metabolism*

Substances

  • Morpholines
  • Neurokinin-1 Receptor Antagonists
  • Receptors, Neurokinin-1
  • Aprepitant