Hydroxyl free radical adduct of deoxyguanosine: sensitive detection and mechanisms of formation

Free Radic Res Commun. 1986;1(3):163-72. doi: 10.3109/10715768609083148.

Abstract

DNA or 2-deoxyguanosine reacts with hydroxyl free radical to form 8-hydroxy-deoxyguanosine (8-OH-dG). We found that 8-OH-dG can be effectively separated from deoxyguanosine by high pressure liquid chromatography and very sensitively detected using electrochemical detection. The sensitivity of electrochemical detection is about one-thousand fold enhanced over optical detection. Utilizing deoxyguanosine in bicarbonate buffer it was found that ferrous ion, but not ferric ion, was effective in forming 8-OH-dG. The hydroxyl free radical scavenging agents, thiourea and ethanol, were very effective in quenching Fe(11) mediated 8-OH-dG formation, but superoxide dismutase had very little effect.

Publication types

  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • 8-Hydroxy-2'-Deoxyguanosine
  • Chromatography, High Pressure Liquid
  • Deoxyguanosine / analogs & derivatives
  • Deoxyguanosine / analysis
  • Deoxyguanosine / metabolism*
  • Electrochemistry
  • Ethanol / pharmacology
  • Free Radical Scavengers
  • Free Radicals
  • Hydroxyl Radical / analysis
  • Hydroxyl Radical / metabolism*
  • Thiourea / pharmacology

Substances

  • Free Radical Scavengers
  • Free Radicals
  • Hydroxyl Radical
  • Ethanol
  • 8-Hydroxy-2'-Deoxyguanosine
  • Deoxyguanosine
  • Thiourea