Estrogen receptor coregulator binding modulators (ERXs) effectively target estrogen receptor positive human breast cancers

Elife. 2017 Aug 8:6:e26857. doi: 10.7554/eLife.26857.

Abstract

The majority of human breast cancer is estrogen receptor alpha (ER) positive. While anti-estrogens/aromatase inhibitors are initially effective, resistance to these drugs commonly develops. Therapy-resistant tumors often retain ER signaling, via interaction with critical oncogenic coregulator proteins. To address these mechanisms of resistance, we have developed a novel ER coregulator binding modulator, ERX-11. ERX-11 interacts directly with ER and blocks the interaction between a subset of coregulators with both native and mutant forms of ER. ERX-11 effectively blocks ER-mediated oncogenic signaling and has potent anti-proliferative activity against therapy-sensitive and therapy-resistant human breast cancer cells. ERX-11 is orally bioavailable, with no overt signs of toxicity and potent activity in both murine xenograft and patient-derived breast tumor explant models. This first-in-class agent, with its novel mechanism of action of disrupting critical protein-protein interactions, overcomes the limitations of current therapies and may be clinically translatable for patients with therapy-sensitive and therapy-resistant breast cancers.

Keywords: E. coli; breast cancer; cancer biology; coagulator binding modulator; coregulators; endocrine therapy; estrogen receptor; mouse.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, N.I.H., Extramural
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Administration, Oral
  • Animals
  • Breast Neoplasms / drug therapy*
  • Cell Line, Tumor
  • Disease Models, Animal
  • Estrogen Receptor Antagonists / administration & dosage
  • Estrogen Receptor Antagonists / metabolism*
  • Heterografts
  • Humans
  • Mice
  • Neoplasm Transplantation
  • Organ Culture Techniques
  • Protein Binding
  • Receptors, Estrogen / metabolism*
  • Signal Transduction / drug effects

Substances

  • Estrogen Receptor Antagonists
  • Receptors, Estrogen