Modulating cellular autophagy for controlled antiretroviral drug release

Nanomedicine (Lond). 2018 Sep;13(17):2139-2154. doi: 10.2217/nnm-2018-0224. Epub 2018 Aug 21.

Abstract

Aim: Pharmacologic agents that affect autophagy were tested for their abilities to enhance macrophage nanoformulated antiretroviral drug (ARV) depots and its slow release.

Methods: These agents included URMC-099, rapamycin, metformin, desmethylclomipramine, 2-hydroxy-β-cyclodextrin (HBC) and clonidine. Each was administered with nanoformulated atazanavir (ATV) nanoparticles to human monocyte-derived macrophages. ARV retention, antiretroviral activity and nanocrystal autophagosomal formation were evaluated.

Results: URMC-099, HBC and clonidine retained ATV. HBC, URMC-099 and rapamycin improved intracellular ATV retention. URMC-099 proved superior among the group in affecting antiretroviral activities.

Conclusion: Autophagy inducing agents, notably URMC-099, facilitate nanoformulated ARV depots and lead to sustained release and improved antiretroviral responses. As such, they may be considered for development as part of long acting antiretroviral treatment regimens.

Keywords: 2-hydroxy-β-cyclodextrin (HBC); URMC-099; autophagy; clonidine; desmethylclomipramine (DMC); long acting slow effective release antiretroviral therapy; metformin; monocyte-derived macrophages; rapamycin.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Anti-HIV Agents / administration & dosage
  • Anti-HIV Agents / chemistry*
  • Anti-HIV Agents / pharmacology
  • Atazanavir Sulfate / administration & dosage
  • Atazanavir Sulfate / chemistry
  • Atazanavir Sulfate / pharmacology*
  • Autophagy / drug effects*
  • Cell Survival / drug effects
  • Clomipramine / administration & dosage
  • Clomipramine / analogs & derivatives
  • Clomipramine / chemistry
  • Clomipramine / pharmacology
  • Clonidine / administration & dosage
  • Clonidine / chemistry
  • Clonidine / pharmacology
  • Drug Carriers / chemistry*
  • Drug Interactions
  • Drug Liberation
  • HIV-1 / drug effects
  • Humans
  • Macrophages / cytology
  • Macrophages / drug effects
  • Macrophages / metabolism
  • Metformin / administration & dosage
  • Metformin / chemistry
  • Metformin / pharmacology
  • Nanoparticles / chemistry*
  • Particle Size
  • Pyridines / administration & dosage
  • Pyridines / chemistry
  • Pyridines / pharmacology
  • Pyrroles / administration & dosage
  • Pyrroles / chemistry
  • Pyrroles / pharmacology
  • Sirolimus / administration & dosage
  • Sirolimus / chemistry
  • Sirolimus / pharmacology
  • Tissue Distribution
  • beta-Cyclodextrins / administration & dosage
  • beta-Cyclodextrins / chemistry
  • beta-Cyclodextrins / pharmacology

Substances

  • Anti-HIV Agents
  • Drug Carriers
  • Pyridines
  • Pyrroles
  • URMC-099
  • beta-Cyclodextrins
  • desmethylclomipramine
  • Atazanavir Sulfate
  • Metformin
  • Clonidine
  • Clomipramine
  • Sirolimus