Anti-quenching NIR-II molecular fluorophores for in vivo high-contrast imaging and pH sensing

Nat Commun. 2019 Mar 5;10(1):1058. doi: 10.1038/s41467-019-09043-x.

Abstract

The contrast and sensitivity of in vivo fluorescence imaging has been revolutionized by molecular fluorophores operating in the second near-infrared window (NIR-II; 1000-1700 nm), but an ongoing challenge is the solvatochromism-caused quenching in aqueous solution for the long-wavelength absorbing fluorophores. Herein, we develop a series of anti-quenching pentamethine cyanine fluorophores that significantly overcome the severe solvatochromism, thus affording stable absorption/emission beyond 1000 nm with up to ~ 44-fold enhanced brightness and superior photostability in aqueous solution. These advantages allow for deep optical penetration (8 mm) as well as high-contrast and highly-stable lymphatic imaging superior to clinical-approved indocyanine green. Additionally, these fluorophores exhibit pH-responsive fluorescence, allowing for noninvasive ratiometric fluorescence imaging and quantification of gastric pH in vivo. The results demonstrate reliable accuracy in tissue as deep as 4 mm, comparable to standard pH electrode method. This work unlocks the potential of anti-quenching pentamethine cyanines for NIR-II biological applications.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Electrodes
  • Female
  • Fluorescent Dyes / administration & dosage*
  • Fluorescent Dyes / chemical synthesis
  • Gastric Acidity Determination / instrumentation
  • Hydrogen-Ion Concentration
  • Injections, Intradermal
  • Lymph Nodes / diagnostic imaging
  • Lymphatic Vessels / diagnostic imaging
  • Mice
  • Mice, Inbred BALB C
  • Mice, Inbred ICR
  • Mice, Nude
  • Models, Animal
  • Optical Imaging / instrumentation
  • Optical Imaging / methods*
  • Phantoms, Imaging
  • Spectroscopy, Near-Infrared / methods
  • Stomach / diagnostic imaging
  • Tissue Distribution

Substances

  • Fluorescent Dyes