Characteristic analysis of continuous new particle formation events in Hefei: A case study of the May Day holiday in China

Ecotoxicol Environ Saf. 2021 Sep 1:220:112329. doi: 10.1016/j.ecoenv.2021.112329. Epub 2021 May 18.

Abstract

Studying the characteristics of new particle formation (NPF) is conducive to exploring the impact of atmospheric particulate matter on the climate, environment, and human health. The particle number size distributions (5.6-560 nm) of aerosols were measured using a fast mobility particle sizer (FMPS) from 1 to 11 May 2019. The clean atmosphere was one of the basic conditions for the occurrence of this continuous new particle formation events. It started between 9:00 and 12:00, and it mainly ended after 20:00. The growth rate (GR) and condensation sink (CS) values in Hefei were 2.98 ± 0.97 nm·h-1 and (3.0 ± 0.4) × 10-2 s-1, respectively. Back trajectory clustering analysis revealed that the mass concentration of the air masses from the southeastern part of Henan Province and the southern part of Anhui Province surrounding the study area were relatively high. The analysis results of the potential source contribution function (PSCF) and the concentration weighted trajectory (CWT) methods show that in addition to local pollution, the long-distance transport of pollutants in the Yangtze River Delta (YRD) greatly contributed to the accumulation modal particulate concentration in Hefei. Moreover, the population affected by PM2.5 during the observation period reached 8.19 × 104, accounting for 1.08% to the total population in Hefei. The premature death cases associated with PM2.5 reached 8.35 × 102. This study is helpful to understand the main influencing factors of consecutive NPF events and the health risks of fine particles.

Keywords: Continuous NPF events; Health risk assessment; Hefei; PM(2.5); Regional transport.

MeSH terms

  • Aerosols / analysis*
  • Air Pollutants / analysis*
  • Air Pollution / analysis*
  • China
  • Environmental Monitoring*
  • Holidays
  • Particulate Matter / analysis*

Substances

  • Aerosols
  • Air Pollutants
  • Particulate Matter