Achieving Superior Cyclability Pouch Cells with Oxygen Vacancy-Moderated P'2/P3 Hybrid Layered Sodium Cathode Materials

ACS Appl Mater Interfaces. 2024 Sep 4;16(35):46216-46225. doi: 10.1021/acsami.4c07264. Epub 2024 Aug 21.

Abstract

Layered P2-type sodium manganese oxide has emerged as a promising cathode candidate for sodium-ion batteries due to its appealing cost-effectiveness and high discharge voltage. However, its practical capacity within the voltage range of 2.0-4.0 V (vs Na+/Na) is relatively low, and its rate capability is hampered by the adverse charge/vacancy ordering during charge/discharge. In this study, a layered P'2/P3 mixed-phase Na0.8-aMn0.675Ni0.225Li0.1O2-x cathode with high (003) crystal plane intensity was designed by introducing oxygen vacancies to P2-structured materials. Aided by these advantages, the hybrid cathode material demonstrates impressive structural and thermal stability and faster Na-ion diffusion kinetics compared to a regular P2 material. Half-cell shows an initial discharge capacity retention of 101 mA h/g at 12 mA/g and 92.25% retention after 500 cycles at 120 mA/g. In combination with a hard carbon anode, the 0.5 A h pouch cell achieved a prevailing capacity retention of 95.2% after 2600 cycles at 36 mA/g. This work opens new dimensions for layered cathode materials with the aim of achieving superior cyclabilities.

Keywords: P′2/P3-type layered oxide cathodes; oxygen vacancy; pouch cell; single-crystalline; sodium-ion batteries.