Recent progress of flexible solid-state supercapacitors: electrodes, electrolytes and practical application

Chemphyschem. 2024 Nov 15:e202400957. doi: 10.1002/cphc.202400957. Online ahead of print.

Abstract

Flexible solid-state supercapacitors (FSSCs) have garnered significant attention due to their advantages, including lightness, adaptability, enhanced safety, and extensive operational potential windows. These features make them highly suitable as energy storage devices for the next generation of portable and flexible electronics. The recent surge in the development and remarkable breakthroughs in novel wearable electronics have further propelled research into FSSCs. Nevertheless, several pressing issues need to be addressed in this field, including synthesizing flexible electrode materials with superior electrochemical energy storage capabilities, enhancing the physicochemical properties of solid gel polymer electrolytes, particularly in extreme environments, and ensuring effective contact between electrodes and gel electrolytes. This paper presents an overview of the latest advancements in FSSCs, focusing on electrode materials and electrolytes. Additionally, it delves into the current challenges and future prospects of FSSCs.

Keywords: Flexible solid-state supercapacitors, Electrode materials, Gel electrolytes, Electrochemical energy storage.